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A high-DPI screenshot setting would be very handy for a high-resolution display such as that in the purported Chromebook Pixel.
 
Here's one trick to make high quality screenshots of Google Chrome OS:
Go to chrome://flags and enable "Force high DPI mode" flag.

As you can see, usability is kinda awful for existing Chromebooks but it might be good for HD TV or upcoming chromebook devices ;)
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